I'd have to go with Lilligant. Lilligant seems frail and weak, but she can be surprisingly deadly in the right hands. And she's just so pretty~!
Discounting Grass-types from the list entirely, I'd probably go with Rayquaza or Gallade. Both of them are awesome, the former being my first experience of being defeated by a wild Pokémon, and the latter being my favorite design in Generation IV, the generation where I had almost lost my connection with Pokémon, due to being ostracized for being a Pokémon junkie.
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